柯长春
副研究员
上海交通大学机械与动力工程学院,博士,副研究员。江西瑞昌人,出生于1983年,2012年毕业于中科院大连化学物理研究所获化学工程专业博士学位。主要从事燃料电池、化工过程系统集成等方面的研究工作。先后主持或参与中国科学院GF科技创新重点部署项目、JK863项目、国家自然科学基金项目等多项。
kechangchun@sjtu.edu.cn
研究方向
(1)燃料电池技术
- 质子交换膜燃料电池技术;
- 基于燃料电池技术的化学电池新体系;
- 高温质子交换膜燃料电池技术;
- 其它先进化学发电技术。
(2)电解池技术
- 二氧化碳电化学还原电解池技术;
- 水电解制氢技术。
项目介绍
- 2015-2017 中国科学院GF科技创新重点部署项目课题“××系统集成与测试评价技术研究”,主任设计师,负责人
- 2015-2017 国家自然科学基金青年项目“面向二电子氧还原的纳米石墨稳定化合金催化剂制备与构效关系研究”,负责人
- 2014-2016 中国科学院GF科技创新基金项目“某原料配制及其产单态氧机理研究”, 负责人
- 2014-2015 中国科学院大连化学物理研究所张存浩院士最高奖基金项目“COIL新型BDP原料规模化制备工艺研究”,负责人
- 2014-2016 大连化学物理研究所博士探索基金课题“BDP制备工艺研究”,负责人
- 2015-2016 中国科学院重点实验室创新基金课题“基于离子液体的无水化产O2(1Δ)反应体系构建与机理研究”,负责人
代表性论文专著
发表SCI论文50余篇,主要论文如下:
- KY Jiang, PP Peng, D Tranca, GS Tong*, Changchun Ke*, CB Lu, J Hu, HW Liang, JT Li, SQ Zhou, E Kymakis, XD Zhuang*, Covalent triazine frameworks and porous carbons: Perspective from an azulene-based case, Macromolecular Rapid Communications, 2022, DOI: 10.1002/marc.202200392
- H Yang, YZ Zhao, ZY Chen, SH Huang, CB Lu, Changchun Ke*, GQ Zhai, JH Zhu, XD Zhuang*, A Narrow Bandgap, Isocyanide-Based Coordination Polymer Framework for Micro-Supercapacitors with AC Line-Filtering Performance, Macromolecular Chemistry and Physics, 2022, 223(10), 2200037
- ZH Yang, KY Jiang, GS Tong, Changchun Ke*, HF Wu, P Liu, JC Zhang, HP Ji, JH Zhu, CB Lu, XD Zhuang*: Copper-involved highly efficient oxygen reduction reaction in both alkaline and acidic media, Chemical Engineering Journal, 2022, 437, 135377.
- W Bao, SH Huang, D Tranca, BX Feng, F Qiu, FR Hernández, Changchun Ke*, S Han, XD Zhuang*: Molecular Engineering of CoII Porphyrins with Asymmetric Architecture for Improved Electrochemical CO2 Reduction, ChemSusChem, 2022, DOI: 10.1002/cssc.202200090
- Y Yuan, YZ Zhao, S Yang, S Han, CB Lu*, HP Ji*, TF Wang, Changchun Ke*, Q Xu, JH Zhu , XD Zhuang: Modulating intramolecular electron and proton transfer kinetics for promoting carbon dioxide conversion, Chemical Communications, 2022, DOI: 10.1039/D1CC06731A
- SH Zhang, KY Jiang, HT Jiang, JH Zhu, HP Ji, CB Lu, LH Zhang, J Li, ZY Chen, Changchun Ke*, XD Zhuang:Pt3Fe nanoparticles triggered high catalytic performance for oxygen reduction reaction in both alkaline and acidic media,ChemElectroChem, 2021, DOI: 10.1002/celc.202101458
- QQ Wan, YY Liu, Changchun Ke*, Y Zhang, WX Jiang, Y Qu, LH Zhang, J Li, J Gui, JB Hou, GF Xia, JW Yin, JL Zhang*: Insight on Performance Degradation of Phthalocyanine Cobalt-Based Gas Diffusion Cathode for Carbon Dioxide Electrochemical Reduction, ACS Sustainable Chemistry & Engineering, 2021, DOI: 10.1021/acssuschemeng.1c07158
- Shu Yuan,Qian Gao,Changchun Ke,Tao Zuo,Junbo Hou,Junliang Zhang: Mesoporous carbon materials for electrochemical energy storage and conversion,ChemElectroChem,2021, DOI: 10.1002/celc.202101182
- Nana Li, Kaiyue Jiang, Fermín Rodríguez-Hernández, Haiyan Mao, Sheng Han,* Xiaobin Fu, jichao Zhang, Chongqing Yang,* Changchun Ke,* Zhuang XD*, Polyarylether-based Two-dimensional Covalent-organic Frameworks with In-plane D-A Structures and Tunable Energy Levels for Energy Storage, Advanced Science, 2021, DOI: 10.1002/advs.202104898
- C. Lu, K. Jiang, D.Tranca, N. Wang, H. Zhu, F. Rodríguez-Hernández, Z. Chen, C. Yang, F. Zhang, Y. Su, Changchun Ke*, J. Zhang, Y.Han, Zhuang XD: Electrochemical reduction of carbon dioxide with nearly 100% carbon monoxide faradaic efficiency from vacancy-stabilized single-atom active sites J. Mater. Chem. A, 2021, DOI: 10.1039/D1TA05990D.
- Wen J, Chen ZY, Han S, Zhu JH, Changchun Ke*, Kymakis E, Zhuang XD: Poly(2-aminoazulene) Filler–Improved PEO-Based Electrolyte for Highly Stable Solid-State Li-Metal Batteries. J Electrochem Soc 2021, 168(3), 090545.
- Ding J, Wu D, Huang S, Lu C, Chen Y, Zhang J, Zhang L, Li J, Changchun Ke*, Tranca D et al: Topological defects involving Fe/N co-doped mesoporous carbon nanosheets as novel electrocatalysts for the oxygen reduction reaction and Zn–air batteries. Nanoscale, 2021,13, 13249-13255
- Wan QQ, He QC, Zhang Y, Zhang LH, Li J, Hou JB, Zhuang XD, Changchun Ke*, Zhang JL: Boosting the Faradaic Efficiency for Carbon Dioxide to Monoxide on a Phthalocyanine Cobalt based Gas Diffusion Electrode to higher than 99% via Microstructure Regulation of Catalyst Layer. Electrochimica Acta, 2021, j.electacta.2021.139023
- Zhuang TJ, Yuan L, Wan QQ, Zhang Y, Li J, Zhang LH, Hou JB, Changchun Ke*, Zhang JL: Investigation on a Novel Direct Liquid Fuel Cell Feeding on Oxalyl Dihydrazide. J Electrochem Soc 2021, 168(3).
- Zhao X, Huang S, Chen Z, Lu C, Han S, Changchun Ke*, Zhu J, Zhang J, DianaTranca, Zhuang X: Carbon nanosheets supporting Ni-N3S single-atom sites for efficient electrocatalytic CO2 reduction. Carbon 2021, 178:488-496.
- Yu TL, Wang YF, Jiang KY, Zhai GQ, Changchun Ke*, Zhang JC, Li JT, Tranca D, Kymakis E, Zhuang XD: Catechol-Coordinated Framework Film-based Micro-Supercapacitors with AC Line Filtering Performance. Chem-Eur J 2021, 27(20):6340-6347.
- Wen YZ, Chen PN, Wang L, Li SY, Wang ZY, Abed J, Mao XN, Min YM, Dinh CT, De Luna P, Changchun Ke et al: Stabilizing Highly Active Ru Sites by Suppressing Lattice Oxygen Participation in Acidic Water Oxidation. J Am Chem Soc 2021, 143(17):6482-6490.
- Wang X, Fu Y, Tranca D, Jiang K, Zhu J, Zhang J, Han S, Changchun Ke, Lu C, Zhuang X: Regulating the Spin State of Nickel in Molecular Catalysts for Boosting Carbon Dioxide Reduction. Acs Appl Energ Mater 2021, 4(3):2891-2898.
- Wang HX, Qiu F, Lu CB, Zhu JH, Changchun Ke*, Han S, Zhuang XD: A Terpyridine-Fe2+-Based Coordination Polymer Film for On-Chip Micro-Supercapacitor with AC Line-Filtering Performance. Polymers 2021, 13(7).
- Ouyang ZP, Tranca D, Zhao YZ, Chen ZY, Fu XB, Zhu JH, Zhai GQ, Changchun Ke*, Kymakis E, Zhuang XD: Quinone-Enriched Conjugated Microporous Polymer as an Organic Cathode for Li-Ion Batteries. Acs Appl Mater Inter 2021, 13(7):9064-9073.
- Liu YP, Wang HX, Liu FR, Kang JL, Qiu F, Changchun Ke, Huang Y, Han S, Zhang F, Zhuang XD: Self-Assembly Approach Towards MoS2-Embedded Hierarchical Porous Carbons for Enhanced Electrocatalytic Hydrogen Evolution. Chem-Eur J 2021, 27(6):2155-2164.
- Jiang PF, Jiang KY, Tranca D, Zhu JH, Qiu F, Changchun Ke, Lu CB, Kymakis E, Zhuang XD: Rational Control of Topological Defects in Porous Carbon for High-Efficiency Carbon Dioxide Conversion. Adv Mater Interfaces 2021, 8(7).
- Huang J, Jiang K, Tranca D, Changchun Ke*, Zhang L, Li J, Li J, Tong G, Kymakis E, Zhuang X: Perovskite oxide and polyazulene–based heterostructure for high–performance supercapacitors. J Appl Polym Sci 2021, 51198.
- Chen ZY, Chen YH, Zhao YZ, Qiu F, Jiang KY, Huang SH, Changchun Ke, Zhu JH, Tranca D, Zhuang XD: B/N-Enriched Semi-Conductive Polymer Film for Micro-Supercapacitors with AC Line-Filtering Performance. Langmuir 2021, 37(7):2523-2531.
- Chen C, Huang J, Mishukova V, Jiang K, Ye X, Lu C, Zhenying Chen, Changchun Ke, Su Y, Li J et al: Mass Transport Behaviors in Graphene and Polyaniline Heterostructure–Based Microsupercapacitors. Advanced Energy & Sustainability Research 2021, 2:2100006.
- Zhu FJ, Luo LX, Wu AM, Wang C, Cheng XJ, Shen SY, Changchun Ke, Yang H, Zhang JL: Improving the High-Current-Density Performance of PEMFC through Much Enhanced Utilization of Platinum Electrocatalysts on Carbon. Acs Appl Mater Inter 2020, 12(23):26076-26083.
- Zhao D, Jiang K, Li J, Zhu X, Changchun Ke, Han S, Kymakis E, Zhuang X: Supercapacitors with alternating current line-filtering performance. BMC Materials 2020, 2(1):3.
- Tu KJ, Zou LY, Yang CQ, Su YZ, Lu CB, Zhu JH, Zhang F, Changchun Ke*, Zhuang XD: Ionic Polyimide Derived Porous Carbon Nanosheets as High-Efficiency Oxygen Reduction Catalysts for Zn-Air Batteries. Chem-Eur J 2020, 26(29):6525-6534.
- Kang JL, Wang MJ, Lu CB, Changchun Ke*, Liu P, Zhu JH, Qiu F, Zhuang XD: Platinum Atoms and Nanoparticles Embedded Porous Carbons for Hydrogen Evolution Reaction. Materials 2020, 13(7).
- Huang JQ, Huang SH, Zhao YZ, Feng BX, Jiang KY, Sun S, Changchun Ke*, Kymakis E, Zhuang XD: Azulene-Based Molecules, Polymers, and Frameworks for Optoelectronic and Energy Applications. Small Methods 2020, 4(10).
- Hou JB, Yang M, Changchun Ke, Zhang JL: Control logics and strategies for air supply in PEM fuel cell engines. Appl Energ 2020, 269.
- Hou JB, Yang M, Changchun Ke, Wei GH, Zhang JL: Optimizing the structural design of a nanocomposite catalyst layer for PEM fuel cells for improving mass-specific power density. Nanoscale 2020, 12(26):13858-13878.
- Hou JB, Yang M, Changchun Ke, Wei GH, Priest C, Qiao Z, Wu G, Zhang JL: Platinum-group-metal catalysts for proton exchange membrane fuel cells: From catalyst design to electrode structure optimization. Energychem 2020, 2(1).
- Han AD, Fu CH, Yan XH, Chen JR, Cheng XJ, Changchun Ke, Hou JB, Shen SY, Zhang JL: Effect of cobalt ion contamination on proton conduction of ultrathin Nafion film. Int J Hydrogen Energ 2020, 45(46):25276-25285.
- Wu AM, Wei GH, Yang F, Xia GF, Yan XH, Shen SY, Zhu FJ, Changchun Ke, Zhang JL: Nitrogen and iodine dual-doped 3D porous graphene as a bi-functional cathode catalyst for Li-O-2 batteries. Electrochim Acta 2019, 318:354-361.
- Wang C, Cheng XJ, Yan XH, Shen SY, Changchun Ke, Wei GH, Zhang JL: Respective Influence of Ionomer Content on Local and Bulk Oxygen Transport Resistance in the Catalyst Layer of PEMFCs with Low Pt Loading. J Electrochem Soc 2019, 166(4):F239-F245.
- Shen SY, Zhang Y, Wei GH, Zhang WS, Yan XH, Xia GF, Wu AM, Changchun Ke, Zhang JL: Li2FeSiO4/C hollow nanospheres as cathode materials for lithium-ion batteries. Nano Res 2019, 12(2):357-363.
- Lin C, Yan XH, Wei GH, Changchun Ke, Shen SY, Zhang JL: Optimization of configurations and cathode operating parameters on liquid-cooled proton exchange membrane fuel cell stacks by orthogonal method. Appl Energ 2019, 253.
- Cheng XJ, Wang C, Wei GH, Yan XH, Shen SY, Changchun Ke, Zhu FJ, Zhang JL: Insight into the Effect of Pore-forming on Oxygen Transport Behavior in Ultra-Low Pt PEMFCs. J Electrochem Soc 2019, 166(14):F1055-F1061.
- Chen JR, Yan XH, Fu CH, Feng Y, Lin C, Li XL, Shen SY, Changchun Ke, Zhang JL: Insight into the Rapid Degradation Behavior of Nonprecious Metal Fe-N-C Electrocatalyst-Based Proton Exchange Membrane Fuel Cells. Acs Appl Mater Inter 2019, 11(41):37779-37786.
- Shen SY, Li F, Luo LX, Guo YG, Yan XH, Changchun Ke, Zhang JL: DMF-Coordination Assisted Electrodeposition of Highly Active PtCo Alloy Catalysts for the Oxygen Reduction Reaction. J Electrochem Soc 2018, 165(2):D43-D49.
- Shen SY, Guo YG, Luo LX, Li F, Li L, Wei GH, Yin JW, Changchun Ke, Zhang JL: Comprehensive Analysis on the Highly Active and Stable PdAu/C Electrocatalyst for Ethanol Oxidation Reaction in Alkaline Media. J Phys Chem C 2018, 122(3):1604-1611.
- Asghar MR, Zhang Y, Wu AM, Yan XH, Shen SY, Changchun Ke, Zhang JL: Preparation of microporous Cellulose/Poly(vinylidene fluoride-hexafluoropropylene) membrane for lithium ion batteries by phase inversion method. J Power Sources 2018, 379:197-205.
- Shen SY, Cheng XJ, Wang C, Yan XH, Changchun Ke, Yin JW, Zhang JL: Exploration of significant influences of the operating conditions on the local O-2 transport in proton exchange membrane fuel cells (PEMFCs). Phys Chem Chem Phys 2017, 19(38):26221-26229.
- Xu XB, Chen WW, Hu DP, Liu ZD, Dai YQ, Changchun Ke, Liu YS, Wang JL, Lv GS, Jin YQ et al: Investigation on Separation Performance of Strongly Swirling Flow Singlet Oxygen Generator. Proc Spie 2015, 9255.
- Liu YS, Chen WW, Wang JL, Xu XB, Liu ZD, Changchun Ke, Guo JW, Zhang SQ, Jin YQ, Sang FT: Research on Reaction Zone Structure of High-press, Gravity-independent, Singlet Oxygen Generator. Proc Spie 2015, 9255.
- Changchun Ke, Chen WW, Xu XB, Wang JL, Liu YS, Jin YQ, Sang FT: Investigation on regeneration of Basic Hydrogen Peroxide by electrochemical methods. Proc Spie 2015, 9255.
- Changchun Ke, Li XJ, Qu SG, Shao ZG, Yi BL: Preparation and properties of Nafion/SiO2 composite membrane derived via in situ sol-gel reaction: size controlling and size effects of SiO2 nano-particles. Polym Advan Technol 2012, 23(1):92-98.
- Changchun Ke, Li J, Li XJ, Shao ZG, Yi BL: Protic ionic liquids: an alternative proton-conducting electrolyte for high temperature proton exchange membrane fuel cells. Rsc Adv 2012, 2(24):8953-8956.
- Changchun Ke, Li X-J, Shen Q, Qu S-G, Shao Z-G, Yi B-L: Investigation on sulfuric acid sulfonation of in-situ sol–gel derived Nafion/SiO2 composite membrane. Int J Hydrogen Energ 2011, 36(5):3606-3613.
- Qu SG, Li XJ, Ke CC, Shao ZG, Yi BL: Experimental and modeling study on water dynamic transport of the proton exchange membrane fuel cell under transient air flow and load change. J Power Sources 2010, 195(19):6629-6636.
专著&章节:
- Qiqi Wan, Changchun Ke*. CO2 Electrochemical Reduction to CO: From Catalysts, Electrodes to Electrolytic Cells and Effect of Operating Conditions, Advanced Electrochemical Materials in Energy Conversion and Storage, CRC Press, 2022
- XiaoJin Li, ChangChun Ke, ShuGuo Qu, Jin Li, ZhiGang Shao, BaoLian Yi. High Temperature PEM Fuel Cells Based on Nafion®/SiO2 Composite Membrane, Energy Storage in the Emerging Era of Smart Grids, Intech Press, 2010
软件版权登记及专利
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荣誉奖励
- 上海市技术发明一等奖,主要完成人
- 上海交通大学首届十大科技进展"高功率密度长寿命燃料电池低铂膜电极技术研发及应用",主要完成人
- 中国科学院重点实验室2015年度“先进青年标兵”
- 中国科学院重点实验室2014年度“先进青年标兵”